TAP (Temporal Analysis of Products) studies of the catalytic conversion of biogas to syngas over Ni/SiO2 catalysts

Hdl Handle:
http://hdl.handle.net/10149/92475
Title:
TAP (Temporal Analysis of Products) studies of the catalytic conversion of biogas to syngas over Ni/SiO2 catalysts
Book Title:
ICHEAP-9: 9TH international conference on chemical and process engineering
Authors:
Olea, M. (Maria); Hodgson, S. N. B. (Simon); Sasaki, T. (Takehiko); Aoki, N. (Nobuaki); Mae, K. (Kazuhiro)
Editors:
Pierucci, S. (Sauro)
Affiliation:
University of Teesside. School of Science and Technology.
Citation:
Olea, M. et al.(2009) 'TAP (Temporal Analysis of Products) studies of the catalytic conversion of biogas to syngas over Ni/SiO2 catalysts', 9th international conference on chemical and process engineering, Rome, Italy, May 10 - 13, in Pierucci, S. (ed) ICHEAP-9: 9TH international conference on chemical and process engineering. AIDIC, pp.7-12.
Publisher:
AIDIC
Conference:
9th international conference on chemical and process engineering, 2009, Rome, Italy, May 10 - 13, 2009.
Issue Date:
May-2009
URI:
http://hdl.handle.net/10149/92475
Abstract:
TAP reactor, a unique transient technique, was used to study the mechanism of the conversion of biogas to syngas over a newly-developed Ni/SiO2 mesoporous catalyst. Single-pulse, alternating pulse, and multipulse TAP experiments were performed at increasing temperatures, from RT to 600 degrees C. Important conclusions about diffusion within the mesoporous catalyst, adsorption of reactant species at the surface of the catalyst, reaction and desorption of reaction products along with the type and lifetime of the intermediate species involved, were achievable through a qualitative and semi-quantitative analysis of the experimental TAP data. These findings will be used to propose an optimal catalysts' formulation for the dry reforming reaction of methane with carbon dioxide.
Type:
Meetings and Proceedings; Book Chapter
Language:
en
Keywords:
TAP reactor; Temporal Analysis of Products; catalytic conversion; biogas; syngas; Ni/SiO2 catalysts
Series/Report no.:
Chemical Engineering Transactions; 17
ISSN:
1974-9791
ISBN:
9788895608013
Rights:
No publisher policy information on http://www.sherpa.ac.uk/romeo/ [Accessed 18/02/2010]
Citation Count:
0 [Web of Science, 18/02/2010]

Full metadata record

DC FieldValue Language
dc.contributor.authorOlea, M. (Maria)en
dc.contributor.authorHodgson, S. N. B. (Simon)en
dc.contributor.authorSasaki, T. (Takehiko)en
dc.contributor.authorAoki, N. (Nobuaki)en
dc.contributor.authorMae, K. (Kazuhiro)en
dc.contributor.editorPierucci, S. (Sauro)en
dc.date.accessioned2010-02-18T10:43:19Z-
dc.date.available2010-02-18T10:43:19Z-
dc.date.issued2009-05-
dc.identifier.isbn9788895608013-
dc.identifier.issn1974-9791-
dc.identifier.urihttp://hdl.handle.net/10149/92475-
dc.description.abstractTAP reactor, a unique transient technique, was used to study the mechanism of the conversion of biogas to syngas over a newly-developed Ni/SiO2 mesoporous catalyst. Single-pulse, alternating pulse, and multipulse TAP experiments were performed at increasing temperatures, from RT to 600 degrees C. Important conclusions about diffusion within the mesoporous catalyst, adsorption of reactant species at the surface of the catalyst, reaction and desorption of reaction products along with the type and lifetime of the intermediate species involved, were achievable through a qualitative and semi-quantitative analysis of the experimental TAP data. These findings will be used to propose an optimal catalysts' formulation for the dry reforming reaction of methane with carbon dioxide.en
dc.language.isoenen
dc.publisherAIDICen
dc.relation.ispartofseriesChemical Engineering Transactionsen
dc.relation.ispartofseries17en
dc.rightsNo publisher policy information on http://www.sherpa.ac.uk/romeo/ [Accessed 18/02/2010]en
dc.subjectTAP reactoren
dc.subjectTemporal Analysis of Productsen
dc.subjectcatalytic conversionen
dc.subjectbiogasen
dc.subjectsyngasen
dc.subjectNi/SiO2 catalystsen
dc.titleTAP (Temporal Analysis of Products) studies of the catalytic conversion of biogas to syngas over Ni/SiO2 catalystsen
dc.typeMeetings and Proceedingsen
dc.typeBook Chapteren
dc.contributor.departmentUniversity of Teesside. School of Science and Technology.en
dc.title.bookICHEAP-9: 9TH international conference on chemical and process engineeringen
dc.identifier.conference9th international conference on chemical and process engineering, 2009, Rome, Italy, May 10 - 13, 2009.en
ref.citationcount0 [Web of Science, 18/02/2010]en
or.citation.harvardOlea, M. et al.(2009) 'TAP (Temporal Analysis of Products) studies of the catalytic conversion of biogas to syngas over Ni/SiO2 catalysts', 9th international conference on chemical and process engineering, Rome, Italy, May 10 - 13, in Pierucci, S. (ed) ICHEAP-9: 9TH international conference on chemical and process engineering. AIDIC, pp.7-12.-
prism.startingPage7-
prism.endingPage12-
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